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In order to grow your collection of Porbles and assemble the best team, you need to capture new Porbles with Capture Scrolls.
Weaken your opponent by depleting its HP to a low level. A Porble with lower health is easier to capture. Defeated Porbles can be caught using Capture Scrolls purchased in the Black Cat Magic Shop with ORB.
See the Items section to learn more about Capture Scrolls.